optimizer for CNEB

Vasp transition state theory tools

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cenwanglai
Posts: 46
Joined: Sun Jun 13, 2010 5:46 am

optimizer for CNEB

Post by cenwanglai »

“We recommend using CG or LBFGS when accurate forces are available. This is essential for evaluating curvatures. For high forces (far from the minimum) or inaccurate forces (close to the minimum) the quick-min or FIRE methods are recommended. These two methods do not rely on curvatures, and tend to be less aggressive, better behaved, but also less efficient than CG/LBFGS. ”

The "minimum" in sentence above does not mean the saddle point? When a CNEB calculation is too close to saddle point, CG/LBFGS is improper, and should be switched to QM?
kai
Posts: 56
Joined: Sun Oct 31, 2010 11:01 pm

Re: optimizer for CNEB

Post by kai »

personally my favorite one is FIRE. use quick min with a small displacement 'maxmove=0.02' for 30 steps until the force is down to ~1ev/A; and then move to more powerful alogrithem with large displacement.
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